Quantum interference between the optical Stark effect and resonant harmonic generation in WS2

Observation of Intervalley Biexcitonic Optical Stark Effect in Monolayer WS2.

Coherent optical driving can effectively modify the properties of electronic valleys in transition metal dichalcogenides. Here, we observe a new type of optical Stark effect in monolayer WS2, one that is mediated by intervalley biexcitons under the blue-detuned driving with circularly polarized light. We find that such helical optical driving not only induces an exciton energy downshift at the ...

Valley-selective optical Stark effect in monolayer WS2.

Breaking space-time symmetries in two-dimensional crystals can markedly influence their macroscopic electronic properties. Monolayer transition metal dichalcogenides (TMDs) are prime examples where the intrinsically broken crystal inversion symmetry permits the generation of valley-selective electron populations, even though the two valleys are energetically degenerate, locked by time-reversal ...

Spatial quantum noise in singly resonant second-harmonic generation.

We study the spatial distribution of quantum noise in singly resonant second-harmonic generation. Calculations are performed below threshold for spatial modulational instability. For parameters for which the intracavity fields are modulationally stable the spatial spectrum shows maximum squeezing at k=0, whereas under conditions of modulational instability we find maximum squeezing at finite wa...

Spatial quantum noise in singly resonant second-harmonic generation: errata.

Interference effects in second-harmonic generation within an optical cavity

An experiment is described that investigates certain interference effects for second-harmonic generation within a resonant cavity. By employing a noncollinear geometry, the phases of two fundamental beams from a frequencystabilized dye laser can be controlled unrestricted by the boundary conditions imposed in an optical cavity containing a KDP crystal and resonant at the second harmonic. The fu...